Catalysis; Electronic, Optical and Magnetic Materials; Ceramics and Composites; Chemistry (all); Surfaces, Coatings and Films; Metals and Alloys; Materials Chemistry; General Chemistry
Résumé :
[en] Waste PLA can be upcycled to metal organic frameworks of potential high value in a one-pot synthesis scheme, where PLA depolymerisation occurs in situ. Three homochiral lactate based frameworks were successfully synthesised and characterised from PLA as a feed source, including ZnBLD. The chiral separation ability of ZnBLD was maintained.
Disciplines :
Ingénierie, informatique & technologie: Multidisciplinaire, généralités & autres
Auteur, co-auteur :
Slater, Benjamin ; Barrer Centre, Department of Chemical Engineering, Imperial College London, London SW7 2AZ, UK. Bradley.ladewig@imperial.ac.uk
Wong, So-On; Barrer Centre, Department of Chemical Engineering, Imperial College London, London, United Kingdom
Duckworth, Andrew; Barrer Centre, Department of Chemical Engineering, Imperial College London, London, United Kingdom
White, Andrew J P ; Department of Chemistry, Imperial College London, Molecular Sciences Research Hub, White City Campus, London, United Kingdom
Hill, Matthew R ; CSIRO Private Bag, Australia
LADEWIG, Bradley Paul ; University of Luxembourg > Faculty of Science, Technology and Medicine (FSTM) > Department of Engineering (DoE) ; Barrer Centre, Department of Chemical Engineering, Imperial College London, London, United Kingdom ; Institute for Micro Process Engineering, Karlsruhe Institute of Technology, Eggenstein-Leopoldshafen, Germany
Co-auteurs externes :
yes
Langue du document :
Anglais
Titre :
Upcycling a plastic cup: one-pot synthesis of lactate containing metal organic frameworks from polylactic acid.
Commonwealth Scientific and Industrial Research Organisation Imperial College London
Subventionnement (détails) :
BDS acknowledges CSIRO and Imperial College London for financial support, and thanks Dr Jason Hallett for discussions on PLA waste. The authors acknowledge Dr Charles Romain for providing PLA cups.
J. D. Watson F. H. C. Crick Nature 1953 171 737 738
S. S. Adams P. Bresloff C. G. Mason J. Pharm. Pharmacol. 1976 28 256 257
O. M. Yaghi G. Li H. Li Nature 1995 378 703
X. Fang B. Zong S. Mao Nanomicro Lett. 2018 10 64
D. Banerjee C. M. Simon S. K. Elsaidi M. Haranczyk P. K. Thallapally Chem 2018 4 466 494
S. Mukherjee A. V. Desai S. K. Ghosh Coord. Chem. Rev. 2018 367 82 126
D. N. Dybtsev A. L. Nuzhdin H. Chun K. P. Bryliakov E. P. Talsi V. P. Fedin K. Kim Angew. Chem., Int. Ed. 2006 45 916 920
C. Zhuo Y. Wen S. Hu T. Sheng R. Fu Z. Xue H. Zhang H. Li J. Yuan X. Chen X. Wu Inorg. Chem. 2017 56 6275 6280
G. Férey C. Mellot-Draznieks C. Serre F. Millange J. Dutour S. Surblé I. Margiolaki Science 2005 309 2040 2042
J. H. Cavka S. Jakobsen U. Olsbye N. Guillou C. Lamberti S. Bordiga K. P. Lillerud J. Am. Chem. Soc. 2008 130 13850 13851
S. R. Miller P. A. Wright C. Serre T. Loiseau J. Marrot G. Ferey Chem. Commun. 2005 3850 3852 10.1039/b506677h
M. Lammert M. T. Wharmby S. Smolders B. Bueken A. Lieb K. A. Lomachenko D. D. Vos N. Stock Chem. Commun. 2015 51 12578 12581
A. F. Ahmad, A. R. Razali and I. S. M. Razelan, Utilization of polyethylene terephthalate (PET) in asphalt pavement: A review, IOP Publishing Ltd, Bristol, 2017
R. Koshti L. Mehta N. Samarth J. Polym. Environ. 2018 26 3520 3529
R. Geyer J. R. Jambeck K. L. Law Sci. Adv. 2017 3 e1700782
Manju P. Kumar Roy A. Ramanan C. Rajagopal Mater. Lett. 2013 106 390 392
W. P. R. Deleu I. Stassen D. Jonckheere R. Ameloot D. E. De Vos J. Mater. Chem. A 2016 4 9519 9525
J. Ren X. Dyosiba N. M. Musyoka H. W. Langmi B. C. North M. Mathe M. S. Onyango Int. J. Hydrogen Energy 2016 41 18141 18146
S.-H. Lo D. Senthil Raja C.-W. Chen Y.-H. Kang J.-J. Chen C.-H. Lin Dalton Trans. 2016 45 9565 9573
J. Yang C. A. Trickett S. B. Alahmadi A. S. Alshammari O. M. Yaghi J. Am. Chem. Soc. 2017 139 8118 8121
H. Y. Lin S. Y. Tsai H. T. Yu C. P. Lin J. Polym. Environ. 2018 26 122 131
J. G. Stark and H. G. Wallace, Chemistry Data Book, Murray, 1982
X. Shi X. Dai Y. Cao J. Li C. Huo X. Wang Ind. Eng. Chem. Res. 2017 56 3887 3894
L. Liu D. Zhang L. An H. Zhang Y. Tian J. Appl. Polym. Sci. 2005 95 719 723
B. Slater Z. Wang S. Jiang M. R. Hill B. P. Ladewig J. Am. Chem. Soc. 2017 139 18322 18327
S.-Y. Zhang L. Wojtas M. J. Zaworotko J. Am. Chem. Soc. 2015 137 12045 12049
