[en] Metal halide perovskites are the first solution processed semiconductors that can compete in their functionality with conventional semiconductors, such as silicon. Over the past several years, perovskite semiconductors have reported breakthroughs in various optoelectronic devices, such as solar cells, photodetectors, light emitting and memory devices, and so on. Until now, perovskite semiconductors face challenges regarding their stability, reproducibility, and toxicity. In this Roadmap, we combine the expertise of chemistry, physics, and device engineering from leading experts in the perovskite research community to focus on the fundamental material properties, the fabrication methods, characterization and photophysical properties, perovskite devices, and current challenges in this field. We develop a comprehensive overview of the current state-of-the-art and offer readers an informed perspective of where this field is heading and what challenges we have to overcome to get to successful commercialization.
Disciplines :
Physics
Author, co-author :
Schmidt-Mende, Lukas; Department of Physics, University of Konstanz, Universitaetsstr. 10, 78457 Konstanz, Germany
Dyakonov, Vladimir; Experimental Physics VI, University of Würzburg, Am Hubland, 97074 Würzburg, Germany
Olthof, Selina; Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
Ünlü, Feray; Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
Trong Lê, Khan Moritz; Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
Mathur, Sanjay; Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
Karabanov, Andrei D.; Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen, 45141 Essen, Germany
Lupascu, Doru C.; Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen, 45141 Essen, Germany
Herz, Laura M.; Clarendon Laboratory, Department of Physics, University of Oxford, Parks Road, Oxford OX1 3PU, United Kingdom ; TUM Institute for Advanced Study, 85748 Garching bei München, Germany
Hinderhofer, Alexander; Institute of Applied Physics, University of Tübingen, Auf der Morgenstelle 10, 72076 Tübingen, Germany
Schreiber, Frank; Institute of Applied Physics, University of Tübingen, Auf der Morgenstelle 10, 72076 Tübingen, Germany
Chernikov, Alexey; Department of Physics, University of Regensburg, 93053 Regensburg, Germany ; Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP) and Würzburg-Dresden Cluster of Excellence ct.qmat, Technische Universität Dresden, 01062 Dresden, Germany
Egger, David A.; Department of Physics, Technical University of Munich, 85748 Garching, Germany
Shargaieva, Oleksandra; Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling,’ Kekulestr. 5, 12489 Berlin, Germany
Cocchi, Caterina; Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling,’ Kekulestr. 5, 12489 Berlin, Germany
Unger, Eva; Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling,’ Kekulestr. 5, 12489 Berlin, Germany
Saliba, Michael; Carl von Ossietzky Universität Oldenburg, Institute of Physics, Carl-von-Ossietzky-Straße 9, 26129 Oldenburg, Germany
Byranvand, Mahdi Malekshahi; Institute for Photovoltaics (ipv), University of Stuttgart, Pfaffenwaldring 47, 70569 Stuttgart, Germany and Helmholtz Young Investigator Group, lEK5-Photovoltaik, Forschungszentrum Jülich, 52425 Jülich, Germany
Kroll, Martin; Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden, 01062 Dresden, Germany
Nehm, Frederik; Department of Physics and Materials Science, University of Luxembourg, Luxembourg, Luxembourg
Leo, Karl; Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden, 01062 Dresden, Germany
Redinger, Alex ; University of Luxembourg > Faculty of Science, Technology and Medicine (FSTM) > Department of Physics and Materials Science (DPHYMS)
Höcker, Julian; Experimental Physics VI, University of Würzburg, Am Hubland, 97074 Würzburg, Germany
Kirchartz, Thomas; IEK5-Photovoltaik, Forschungszentrum Jülich, 52425 Jülich, Germany and Faculty of Engineering and CENIDE, University of Duisburg-Essen, Carl-Benz-Str. 199, 47057 Duisburg, Germany
Warby, Jonathan; Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
Gutierrez-Partida, Emilio; Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
Neher, Dieter; Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
Stolterfoht, Martin; Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
Würfel, Uli; Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany ; Department of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstraße 2, 79110 Freiburg, Germany
Unmüssig, Moritz; Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany ; Department of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstraße 2, 79110 Freiburg, Germany
Herterich, Jan; Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany ; Department of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstraße 2, 79110 Freiburg, Germany
Baretzky, Clemens; Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany ; Department of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstraße 2, 79110 Freiburg, Germany
Mohanraj, John; Applied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth, 95440 Bayreuth, Germany
Thelakkat, Mukundan; Applied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth, 95440 Bayreuth, Germany ; Bavarian Polymer Institute, University of Bayreuth, 95440 Bayreuth, Germany
Maheu, Clément; Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
Jaegermann, Wolfram; Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
Mayer, Thomas; Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
Yang, Fengjiu; Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells, 12489 Berlin, Germany
Albrecht, Steve; Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells, 12489 Berlin, Germany ; Technical University Berlin, Faculty IV, Electrical Engineering and Computer Science, 10587 Berlin, Germany
Riedl, Thomas; Institute of Electronic Devices, University of Wuppertal, 42119 Wuppertal, Germany ; Wuppertal Center for Smart Materials and Systems, University of Wuppertal, 42119 Wuppertal, Germany
Fakharuddin, Azhar; Department of Physics, University of Konstanz, Universitaetsstr. 10, 78457 Konstanz, Germany
Vasilopoulou, Maria; Institute of Nanoscience and Nanotechnology, National Center for Scientific Research Demokritos, 15341 Agia Paraskevi, Attica, Greece
Vaynzof, Yana; Integrated Center for Applied Physics and Photonic Materials (IAPP) and Center for Advancing Electronics Dresden (cfaed), Technische Universität Dresden, Nöthnitzer Straße 61, 01187 Dresden, Germany
Moia, Davide; Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569 Stuttgart, Germany
Maier, Joachim; Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569 Stuttgart, Germany
Franckevičius, Marius; Department of Molecular Compound Physics, Center for Physical Sciences and Technology (FTMC), Saul˙etekio Avenue 3, Vilnius LT-10257, Lithuania
Gulbinas, Vidmantas; Department of Molecular Compound Physics, Center for Physical Sciences and Technology (FTMC), Saul˙etekio Avenue 3, Vilnius LT-10257, Lithuania
Kerner, Ross A.; Department of Electrical Engineering, Princeton University, Princeton, New Jersey 08544, USA
Zhao, Lianfeng; Department of Electrical Engineering, Princeton University, Princeton, New Jersey 08544, USA
Rand, Barry P.; Department of Electrical Engineering, Princeton University, Princeton, New Jersey 08544, USA ; Andlinger Center for Energy and the Environment, Princeton University, Princeton, New Jersey 08544, USA
Glück, Nadja; Department of Chemistry, Ludwig-Maximilians-University Munich, Butenandtstr. 5-13, 81377 Munich, Germany
Bein, Thomas; Department of Chemistry, Ludwig-Maximilians-University Munich, Butenandtstr. 5-13, 81377 Munich, Germany
Matteocci, Fabio; CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor Vergata, Roma 00133, Italy
Castriotta, Luigi Angelo; CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor Vergata, Roma 00133, Italy
Di Carlo, Aldo; CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor Vergata, Roma 00133, Italy ; LASE—Laboratory for Advanced Solar Energy, National University of Science and Technology MISiS, 119049 Moscow, Russia
Scheffler, Matthias; Physics Department and IRIS Adlershof, Humboldt-Universität zu Berlin, Zum Großen Windkanal 2, 12489 Berlin, Germany ; Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, 14195 Berlin, Germany
Draxl, Claudia; Physics Department and IRIS Adlershof, Humboldt-Universität zu Berlin, Zum Großen Windkanal 2, 12489 Berlin, Germany ; Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, 14195 Berlin, Germany
