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First law of quantum thermodynamics in a driven open two-level system ; Chenu, Aurélia in Physical Review. A (2021) Assigning the variations of internal energy into heat or work contributions is a challenging task due to the fact that these properties are trajectory dependent. A number of proposals have been put ... [more ▼] Assigning the variations of internal energy into heat or work contributions is a challenging task due to the fact that these properties are trajectory dependent. A number of proposals have been put forward for open quantum systems following an arbitrary dynamics. We here focus on nonequilibrium thermodynamics of a two-level system and explore in addition to the conventional approach, two definitions motivated by either classical work or heat in which the driving Hamiltonian or the trajectory itself, respectively, are used to set up a reference basis. We first give the thermodynamic properties for an arbitrary dynamics and illustrate the results on the Bloch sphere. Then, we solve the particular example of a periodically driven qubit interacting with a dissipative and decoherence bath. Our results illustrate the trajectory-dependent character of heat and work and how contributions originally assigned to dissipation in the Lindblad equation can become a coherent part assigned to work. [less ▲] Detailed reference viewed: 46 (2 UL)Quantum bath statistics tagging ; Cavina, Vasco ; in Physical Review. A (2019) The possibility of discriminating the statistics of a thermal bath using indirect measurements performed on quantum probes is presented. The scheme relies on the fact that, when weakly coupled with the ... [more ▼] The possibility of discriminating the statistics of a thermal bath using indirect measurements performed on quantum probes is presented. The scheme relies on the fact that, when weakly coupled with the environment of interest, the transient evolution of the probe toward its final thermal configuration is strongly affected by the fermionic or bosonic nature of the bath excitations. Using figures of merit taken from quantum metrology such as the Holevo-Helstrom probability of error and the quantum Chernoff bound, we discuss how to achieve the greatest precision in this statistics tagging procedure, analyzing different models of probes and different initial preparations and by optimizing over the time of exposure of the probe. [less ▲] Detailed reference viewed: 43 (0 UL)Rydberg crystallization detection by statistical means ; Schmidt, Thomas ; in Physical Review. A (2012), 86 We investigate an ensemble of atoms which can be excited into a Rydberg state. Using a disordered quantum Ising model, we perform a numerical simulation of the experimental procedure and calculate the ... [more ▼] We investigate an ensemble of atoms which can be excited into a Rydberg state. Using a disordered quantum Ising model, we perform a numerical simulation of the experimental procedure and calculate the probability distribution function $P(M)$ to create a certain number of Rydberg atoms $M$, as well as their pair-correlation function. Using the latter, we identify the critical interaction strength above which the system undergoes a phase transition to a Rydberg crystal. We then show that this phase transition can be detected using $P(M)$ alone. [less ▲] Detailed reference viewed: 86 (1 UL)Rumpling of LiF(001) surface from fast atom diffraction ; ; et al in Physical Review. A (2010), 82(6), 062902 Quantum diffraction of fast atoms scattered from the topmost layer of surfaces under grazing angles of incidence can be employed for the analysis of detailed structural properties of insulator surfaces ... [more ▼] Quantum diffraction of fast atoms scattered from the topmost layer of surfaces under grazing angles of incidence can be employed for the analysis of detailed structural properties of insulator surfaces. From comparison of measured and calculated diffraction patterns we deduce the rumpling of the topmost surface layer of LiF(001) (i.e., an inward shift of Li(+) ions with respect to F(-) ions). The effect of thermal vibrations on the measurement of rumpling is accounted for by ab initio calculations of the mean-square vibrational amplitudes of surface ions. At room temperature this leads to a reduction of the apparent rumpling by 0.008 angstrom. We then obtain a rumpling of ( 0.05 +/- 0.04) angstrom, which improves its accuracy achieved in previous work. [less ▲] Detailed reference viewed: 133 (3 UL)Expansion of a Fermi cloud in the BCS-BEC crossover Diana, Giovanni ; ; in Physical Review. A (2006), 73(6), 065601 We study the free expansion of a dilute two-component Fermi gas with attractive interspecies interaction in the BCS-BEC crossover. We apply a time-dependent parameter-free density-functional theory by ... [more ▼] We study the free expansion of a dilute two-component Fermi gas with attractive interspecies interaction in the BCS-BEC crossover. We apply a time-dependent parameter-free density-functional theory by using two choices of the equation of state: an analytic formula based on Monte Carlo data and the mean-field equation of state resulting from the extended BCS equations. The calculated axial and transverse radii and the aspect ratio of the expanding cloud are compared to experimental data on vapors of 6 Li atoms. Remarkably, the mean-field theory shows a better agreement with the experiments than the theory based on the Monte Carlo equation of state. Both theories predict a measurable dependence of the aspect ratio on expansion time and on scattering length. [less ▲] Detailed reference viewed: 146 (1 UL)Overdamping by weakly coupled environments Esposito, Massimiliano ; in Physical Review. A (2005), 72(6), Detailed reference viewed: 35 (1 UL)Liouville master equation for multielectron dynamics: Neutralization of highly charged ions near a LiF surface Wirtz, Ludger ; ; et al in Physical Review. A (2003), 67(1), We present a simulation of the neutralization of highly charged ions in front of a lithium fluoride surface including the close-collision regime above the surface. The present approach employs a Monte ... [more ▼] We present a simulation of the neutralization of highly charged ions in front of a lithium fluoride surface including the close-collision regime above the surface. The present approach employs a Monte Carlo solution of the Liouville master equation for the joint probability density of the ionic motion and the electronic population of the projectile and the target surface. It includes single as well as double particle-hole (de)excitation processes and incorporates electron correlation effects through the conditional dynamics of population strings. The input in terms of elementary one- and two-electron transfer rates is determined from classical trajectory Monte Carlo calculations as well as quantum-mechanical Auger calculations. For slow projectiles and normal incidence, the ionic motion depends sensitively on the interplay between image acceleration towards the surface and repulsion by an ensemble of positive hole charges in the surface ("trampoline effect"). For Ne10+ we find that image acceleration is dominant and no collective backscattering high above the surface takes place. For grazing incidence, our simulation delineates the pathways to complete neutralization. In accordance with recent experimental observations, most ions are reflected as neutral or even as singly charged negative particles, irrespective of the charge state of the incoming ions. [less ▲] Detailed reference viewed: 139 (0 UL)Potential-energy surfaces for charge exchange between singly charged ions and a LiF surface Wirtz, Ludger ; ; et al in Physical Review. A (2003), 68(3), We analyze the adiabatic potential-energy surfaces relevant for neutralization of singly charged ions in slow vertical incidence onto a lithium fluoride surface. The surface is represented by a cluster of ... [more ▼] We analyze the adiabatic potential-energy surfaces relevant for neutralization of singly charged ions in slow vertical incidence onto a lithium fluoride surface. The surface is represented by a cluster of varying size augmented by point charges of alternating sign in order to include the proper Madelung potential of the ionic crystal. Our calculation proceeds on the multiconfiguration self-consistent-field and multireference configuration-interaction levels. Size-consistency corrections based on the Davidson correction and multireference averaged quadratic coupled cluster methods are included as well. We emphasize the importance of a proper treatment of electron correlation signifying the polarization of the surrounding cluster environment in ab initio calculations of charge transfer at surfaces. From the topology of the surfaces, in particular the existence or absence of avoided crossings (or, more generally, conical intersections), qualitative predictions for the neutralization process can be made. The comparative analysis of potential curves for H+, C+, S+, and Ne+ projectiles provides an explanation for the recently observed threshold behavior for potential sputtering. [less ▲] Detailed reference viewed: 97 (0 UL)Hollow-ion formation in microcapillaries ; Wirtz, Ludger ; et al in Physical Review. A (2001), 64(4), Transmission of highly charged ions through microcapillaries is studied theoretically by a classical trajectory simulation. The interaction of highly charged ions with the internal surface of the ... [more ▼] Transmission of highly charged ions through microcapillaries is studied theoretically by a classical trajectory simulation. The interaction of highly charged ions with the internal surface of the capillary is treated within the framework of dielectric-response theory. The simulation is based on the classical over-the-barrier model modified for open cylindrical surfaces. The multielectron evolution and relaxation is taken into account as a stochastic event sequence. We consider N6+ and Ne10+ with an energy of 2.1 keV/amu passing through a metallic microcapillary of Ni. We analyze the distance of closest approach. the angular distribution, and the distribution of the mean occupation numbers of n shells of highly charged ions. We find the resulting charge state distribution of transmitted projectiles in good agreement with recent measurements. Implications for nanotube targets will be discussed. [less ▲] Detailed reference viewed: 106 (1 UL)Charge-state evolution of highly charged ions transmitted through microcapillaries ; Wirtz, Ludger ; et al in Physical Review. A (2000), 61(2), The charge-state evolution of highly charged ions transmitted through microcapillaries is studied theoretically by a classical trajectory Monte Carlo simulation.: The interaction of highly charged ions ... [more ▼] The charge-state evolution of highly charged ions transmitted through microcapillaries is studied theoretically by a classical trajectory Monte Carlo simulation.: The interaction of highly charged ions with the internal surface of the capillary is treated within the framework of dielectric response theory. We analyze the distance of closest approach and the angular distributions of the highly charged ions at the exit of the microcapillary. We find the charge-state fraction of transmitted N6+ projectiles, in: good agreement with first measurements. Moreover, our calculations indicate that grazing collisions with the microcapillary surface hold the promise of direct observation of charge transfer and hollow-atom formation at a large distance from the surface. [less ▲] Detailed reference viewed: 112 (8 UL) |
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