Neutron study of magnetic correlations in rare-earth-free Mn-Bi magnets

in Physical Review Materials (2021), 5

We report the results of an unpolarized small-angle neutron scattering (SANS) study on Mn-Bi-based rare-earth-free permanent magnets. The magnetic SANS cross section is dominated by long-wavelength ... [more ▼]

We report the results of an unpolarized small-angle neutron scattering (SANS) study on Mn-Bi-based rare-earth-free permanent magnets. The magnetic SANS cross section is dominated by long-wavelength transversal magnetization fluctuations and has been analyzed in terms of the Guinier-Porod model and the distance distribution function. This provides the radius of gyration which, in the remanent state, ranges between about $220-240 \, \mathrm{nm}$ for the three different alloy compositions investigated. Moreover, computation of the distance distribution function in conjunction with results for the so-called $s$-parameter obtained from the Guinier-Porod model indicate that the magnetic scattering of a Mn$_{45}$Bi$_{55}$ sample has its origin in slightly shape-anisotropic structures. [less ▲]

Magnetic Guinier law

in IUCrJ (2020), 7

Small-angle scattering of x-rays and neutrons is a routine method for the determination of nanoparticle sizes. The so-called Guinier law represents the low-q approximation for the small-angle scattering ... [more ▼]

Small-angle scattering of x-rays and neutrons is a routine method for the determination of nanoparticle sizes. The so-called Guinier law represents the low-q approximation for the small-angle scattering curve from an assembly of particles. The Guinier law has originally been derived for nonmagnetic particle-matrix-type systems, and it is successfully employed for the estimation of particle sizes in various scientific domains (e.g., soft matter physics, biology, colloidal chemistry, materials science). An important prerequisite for it to apply is the presence of a discontinuous interface separating particles and matrix. Here, we introduce the Guinier law for the case of magnetic small-angle neutron scattering (SANS) and experimentally demonstrate its applicability for the example of nanocrystalline cobalt. It is well- known that the magnetic microstructure of nanocrystalline ferromagnets is highly nonuniform on the nanometer length scale and characterized by a spectrum of continuously varying long-wavelength magnetization fluctuations, i.e., these systems do not manifest sharp interfaces in their magnetization profile. The magnetic Guinier radius depends on the applied magnetic field, on the magnetic interactions (exchange, magnetostatics), and on the magnetic anisotropy-field radius, which characterizes the size over which the magnetic anisotropy field is coherently aligned into the same direction. In contrast to the nonmagnetic conventional Guinier law, the magnetic version can be applied to fully dense random-anisotropy-type ferromagnets. [less ▲]

Evidence for the formation of nanoprecipitates with magnetically disordered regions in bulk Ni50Mn45In5 Heusler alloys

in Physical Review. B, Condensed Matter and Materials Physics (2019), 99

Field-Induced Spin Helix Chirality in Nanocrystalline Ho

Poster (2014, November)